Exasperated means worn out by something that keeps going wrong. An exasperated sigh, exasperated with him, growing exasperated.
The repetition is what makes it — you are exasperated by the fourth time, not the first — and it is tiredness as much as anger. It sits between annoyed and furious and it usually shows in the voice rather than in what is said.
1adjectiveexasperatedWorn out by something that keeps going wrong.
“After the printer jammed for the third time, she threw up her hands, completely exasperated.”
exasperated is a state of irritation.